Anthropogenic impact on Antarctic surface mass balance, currently masked by natural variability, to emerge by mid-century

Global and regional climate models robustly simulate increases in Antarctic surface mass balance (SMB) during the twentieth and twenty-first centuries in response to anthropogenic global warming. Despite these robust model projections, however, observations indicate that there has been no significant change in Antarctic SMB in recent decades. We show that this apparent discrepancy between models and observations can be explained by the fact that the anthropogenic climate change signal during the second half of the twentieth century is small compared to the noise associated with natural climate variability. Using an ensemble of 35 global coupled climate models to separate signal and noise, we find that the forced SMB increase due to global warming in recent decades is unlikely to be detectable as a result of large natural SMB variability. However, our analysis reveals that the anthropogenic impact on Antarctic SMB is very likely to emerge from natural variability by the middle of the current century, thus mitigating future increases in global sea level

Comment on “Tropospheric Temperature Response to Stratospheric Ozone Recovery in the 21st Century” by Hu et al. (2011)

Stratospheric ozone recovery is expected to figure prominently in twenty-first century climate change. In a recent paper, Hu et al. (2011) argue that one impact of ozone recovery will be to enhance the warming of the surface-troposphere system produced by increases in well-mixed greenhouse gases. Furthermore, this enhanced warming would be strongest in the Northern Hemisphere, which is surprising since previous studies have consistently shown the effects of stratospheric ozone changes to be most pronounced in the Southern Hemisphere. Hu et al. (2011) base their claims largely on differences in the simulated temperature change between two groups of CMIP3 (Coupled Model Intercomparison Project 3) climate models, one group which included stratospheric ozone recovery in its twenty-first century simulations and a second group which did not. Both groups of models were forced with the same increases in well-mixed greenhouse gases according to the A1B emissions scenario. In the current work, we compare the surface temperature responses of the same two groups of models in a different experiment in which atmospheric CO2 was increased by 1% per year until doubling. We find remarkably similar differences in the simulated surface temperature change between the two sets of models as Hu et al. (2011) found for the A1B experiment, suggesting that the enhanced warming which they attribute to stratospheric ozone recovery is actually a reflection of different responses of the two model groups to greenhouse gas forcing

Large Cancellation, Due to Ozone Recovery, of Future Southern Hemisphere Atmospheric Circulation Trends

The role of stratospheric ozone recovery in the Southern Hemisphere climate system, in the coming decades, is examined by contrasting two 10-member ensembles of Community Atmospheric Model (CAM3) integrations, over the period 2000–2060. Model integrations in the first ensemble are conducted with a complete set of forcings: greenhouse gas concentrations from the A1B scenario, SSTs from corresponding ocean-atmosphere coupled model integrations, and ozone starting with severe depletion over the South Pole and recovering by mid-century. The integrations in the second ensemble are very similar to the first, except that only the transient ozone forcing is specified, and all other forcings are kept at year 2000 levels. Specifying ozone recovery in isolation allows us to determine unambiguously how it impacts the atmospheric circulation. We find that, in DJF, most key indices of atmospheric circulation show significant trends in the second ensemble, due to the closing of the ozone hole. In the first ensemble, however, trends are found to be statistically insignificant for nearly all key circulation indices. This suggests that ozone recovery will result in a nearly complete cancellation (and possible reversal) of the atmospheric circulation effects associated with increasing greenhouse gases, in Southern Hemisphere summer, over the coming half century

The Antarctic Atmospheric Energy Budget. Part I: Climatology and Intraseasonal-to-Interannual Variability

The authors present a new, observationally based estimate of the atmospheric energy budget for the Antarctic polar cap (the region poleward of 70°S). This energy budget is constructed using state-of-the-art reanalysis products from ECMWF [the ECMWF Interim Re-Analysis (ERA-Interim)] and Clouds and the Earth's Radiant Energy System (CERES) top-of-atmosphere (TOA) radiative fluxes for the period 2001–10. The climatological mean Antarctic energy budget is characterized by an approximate balance between the TOA net outgoing radiation and the horizontal convergence of atmospheric energy transport, with the net surface energy flux and atmospheric energy storage generally being small in comparison. Variability in the energy budget on intraseasonal-to-interannual time scales bears a strong signature of the southern annular mode (SAM), with El Niño–Southern Oscillation (ENSO) having a smaller impact. The energy budget framework is shown to be a useful alternative to the SAM for interpreting surface climate variability in the Antarctic region

The Antarctic Atmospheric Energy Budget. Part II: The Effect of Ozone Depletion and its Projected Recovery

In this study we continue our investigation of the atmospheric energy budget of the Antarctic polar cap (the region poleward of 70°S) using integrations of the Whole Atmosphere Community Climate Model from the year 1960 to 2065. In agreement with observational data, we find that the climatological mean net top-of-atmosphere (TOA) radiative flux is primarily balanced by the horizontal energy flux convergence over the polar cap. On interannual timescales, changes in the net TOA radiative flux are also primarily balanced by changes in the energy flux convergence, with the variability in both terms significantly correlated with the Southern Annular Mode (SAM); positive and negative correlations, respectively. On multidecadal timescales, twentieth century stratospheric ozone depletion produces a negative trend in the net TOA radiative flux due to a decrease in the absorbed solar radiation within the atmosphere-surface column. The negative trend in the net TOA radiative flux is balanced by a positive trend in energy flux convergence, primarily in austral summer. This negative (positive) trend in the net TOA radiation (energy flux convergence) occurs despite a positive trend in the SAM, suggesting that the effects of the SAM on the energy budget are overwhelmed by the direct radiative effects of ozone depletion. In the twenty-first century, ozone recovery is expected to reverse the negative trend in the net TOA radiative flux, which would then, again, be balanced by a decrease in the energy flux convergence. Therefore, over the next several decades, ozone recovery will, in all likelihood, mask the effect of GHG warming on the Antarctic energy budget

Timing and seasonality of the United States ‘warming hole’

The United States ‘warming hole’ is a region in the southeast/central U.S. where observed long-term surface temperature trends are insignificant or negative. We investigate the roles of anthropogenic forcing and internal variability on these trends by systematically examining observed seasonal temperature trends over all time periods of at least 10 years during 1901–2015. Long-term summer cooling in the north central U.S. beginning in the 1930s reflects the recovery from the anomalously warm ‘Dust Bowl’ of that decade. In the northeast and southern U.S., significant summertime cooling occurs from the early 1950s to the mid 1970s, which we partially attribute to increasing anthropogenic aerosol emissions (median fraction of the observed temperature trends explained is 0.69 and 0.17, respectively). In winter, the northeast and southern U.S. cool significantly from the early 1950s to the early 1990s, but we do not find evidence for a significant aerosol influence. Instead, long-term phase changes in the North Atlantic Oscillation contribute significantly to this cooling in both regions, while the Pacific Decadal Oscillation also contributes significantly to southern U.S. cooling. Rather than stemming from a single cause, the U.S. warming hole reflects both anthropogenic aerosol forcing and internal climate variability, but the dominant drivers vary by season, region, and time period

Temperature and precipitation extremes in the United States: Quantifying the responses to anthropogenic aerosols and greenhouse gases

Changes in extreme temperatures, heat waves, heavy rainfall events, and precipitation frequency can have adverse impacts on human health, air quality, agricultural productivity, and water resources. Using the aerosol only (AER) and greenhouse gas only (GHG) "single forcing" simulations (3 ensemble members each) from the GFDL CM3 chemistry-climate model, we investigate aerosol- versus greenhouse gas-induced changes in high temperature and precipitation extremes over the United States. We identify changes in these events from 1860 to 2005 and the associated large-scale dynamical conditions. Small changes in these extremes in the "all forcing" simulations reflect cancellations between the individual, opposite-signed effects of increasing anthropogenic aerosols and greenhouse gases. In AER, aerosols lead to lower extreme high temperatures and fewer warm spells over the western US (-2.1 K regional average; -20 days/year) and over the central and northeast US (-1.5 K; -12 days/year). In GHG, a similar but opposite-signed response pattern occurs (+2.7 K and +14 days/year over the western US; +2.5 K and +10 days/year in the central and northeast US). The similar spatial response patterns in AER versus GHG suggest a preferred regional mode of response that is largely independent of the regional distribution of the forcing agent. The influence of both greenhouse gases and aerosols on extreme high temperature is weakest in the southeast US, collocated with the observed "warming hole". No statistically significant change occurs in AER, and a warming of only +1.8 K occurs in GHG. Warming in this region continues to be muted over the 21st century under the RCP 8.5 scenario, with increases in extreme temperatures more than 1 K smaller than elsewhere. Aerosols induce decreases in the number of days per year with at least 10mm of precipitation (R10mm) over the eastern US in summer and winter and over the southern US in spring of roughly 1 day/year. In contrast, greenhouse gases induce increases in R10mm over the eastern US in winter (+0.8 days/year), the northern and central US during spring (+1 day/year), and the southeast US during summer (+0.5 days/year), but decreases over the northeast US in summer (-0.2 days/year). In RCP 8.5, the patterns of extreme temperature and precipitation associated with greenhouse gas forcing dominate

Rapid Screening of Alicyclobacillus acidoterrestris Spoilage of Fruit Juices by Electronic Nose: A Confirmation Study

Early screening of Alicyclobacillus spp. in fruit juices is a major applicative goal for the food industry, since juice contamination can lead to considerable loss of quality, and subsequently, to economic damages for juice producers. This paper presents an accurate study to assess and confirm the EOS507 electronic nose’s (EN) ability of diagnosing Alicyclobacillus acidoterrestris spoilage in artificially contaminated fruit juices. The authors experimental results have shown that the EOS507 can early identify, just after 24 hours from inoculation, contaminated orange and pear juices with an excellent classification rate close to 90% and with a detection threshold as low as 103 cfu/ml. In apple juice the detection threshold was about 105 cfu/ml, thus requiring longer incubation times (72 hours). PLS regression of EOS507 data can be also used to predict with fair accuracy the colony-forming units concentration of the bacteria. These results were supported by the GC/MS/MS measurements of specific chemical markers, such as guaiacol

Local and Remote Mean and Extreme Temperature Response to Regional Aerosol Emissions Reductions

The climatic implications of regional aerosol and precursor emissions reductions implemented to protect human health are poorly understood. We investigate the mean and extreme temperature response to regional changes in aerosol emissions using three coupled chemistryclimate models: NOAA GFDL CM3, NCAR CESM1, and NASA GISS-E2. Our approach contrasts a long present-day control simulation from each model (up to 400 years with perpetual year 2000 or 2005 emissions) with 14 individual aerosol emissions perturbation simulations (160240 years each). We perturb emissions of sulfur dioxide (SO2) and/or carbonaceous aerosol within six world regions and assess the statistical significance of mean and extreme temperature responses relative to internal variability determined by the control simulation and across the models. In all models, the global mean surface temperature response (perturbation minus control) to SO2 and/or carbonaceous aerosol is mostly positive (warming) and statistically significant and ranges from +0.17 K (Europe SO2) to -0.06 K (US BC). The warming response to SO2 reductions is strongest in the US and Europe perturbation simulations, both globally and regionally, with Arctic warming up to 1 K due to a removal of European anthropogenic SO2 emissions alone; however, even emissions from regions remote to the Arctic, such as SO2 from India, significantly warm the Arctic by up to 0.5 K. Arctic warming is the most robust response across each model and several aerosol emissions perturbations. The temperature response in the Northern Hemisphere midlatitudes is most sensitive to emissions perturbations within that region. In the tropics, however, the temperature response to emissions perturbations is roughly the same in magnitude as emissions perturbations either within or outside of the tropics. We find that climate sensitivity to regional aerosol perturbations ranges from 0.5 to 1.0 K (W m(exp -2))(exp -1) depending on the region and aerosol composition and is larger than the climate sensitivity to a doubling of CO2 in two of three models. We update previous estimates of regional temperature potential (RTP), a metric for estimating the regional temperature responses to a regional emissions perturbation that can facilitate assessment of climate impacts with integrated assessment models without requiring computationally demanding coupled climate model simulations. These calculations indicate a robust regional response to aerosol forcing within the Northern Hemisphere midlatitudes, regardless of where the aerosol forcing is located longitudinally. We show that regional aerosol perturbations can significantly increase extreme temperatures on the regional scale. Except in the Arctic in the summer, extreme temperature responses largely mirror mean temperature responses to regional aerosol perturbations through a shift of the temperature distributions and are mostly dominated by local rather than remote aerosol forcing

Single crystal diamond membranes for nanoelectronics

© 2018 The Royal Society of Chemistry. Single crystal, nanoscale diamond membranes are highly sought after for a variety of applications including nanophotonics, nanoelectronics and quantum information science. However, so far, the availability of conductive diamond membranes has remained an unreachable goal. In this work we present a complete nanofabrication methodology for engineering high aspect ratio, electrically active single crystal diamond membranes. The membranes have large lateral directions, exceeding ∼500 × 500 μm2 and are only several hundreds of nanometers thick. We further realize vertical single crystal p-n junctions made from the diamond membranes that exhibit onset voltages of ∼10 V and a current of several mA. Moreover, we deterministically introduce optically active color centers into the membranes, and demonstrate for the first time a single crystal nanoscale diamond LED. The robust and scalable approach to engineer the electrically active single crystal diamond membranes offers new pathways for advanced nanophotonic, nanoelectronic and optomechanical devices employing diamond